Research Areas

Nanophotonic Materials and Devices : Plasmonics

Caltech People: Prof. Harry Atwater (APh), Dr. Henri Lezec, Dr. Domenico Pacifici, Julie Biteen, Jennifer Dionne, Carrie Ross, Luke Sweatlock

Collaborators: Prof. Albert Polman, Hans Mertens (AMOLF)


Plasmonics:

Light can be localized and manipulated in appropriately designed metallic and metallodielectric nanoparticle array structures. In particular, interesting phenomena occur near the plasmon frequency where optical extinction is resonantly enhanced, and at the plasma frequency where the real part of the dielectric constant changes sign. Due to their high reflection and absorption coefficients, metal structures have been generally overlooked as elements to guide, focus and switch light at visible and infrared wavelengths. However at the nanoscale the intriguing guiding and refractive properties of metal structures can be realized since the metal components become semitransparent due to their small size.


Emerging Research Areas:

1. Plasmonic Waveguides

The scaling of optical devices and components to their ultimate size limits will require that electromagnetic energy be guided on a scale below the diffraction limit and that information be guided around sharp corners with nanometer-scale radii of curvature. Plasmon waveguides are periodic chain arrays of metal nanoparticles which can localize light in guided modes whose size is a few percent of the optical wavelength. Such waveguides can enable efficient power transfer around sharp corners and may form the basis for nanoscale all-optical switches.


Click on images to stream FDTD movies. Downloading is available below.

Longitudinal Mode Propagation in Spherical Particles


Download 5.5MB, Quicktime Format



Transverse Mode Propagation in Spheroidal Particles

Notice the negative phase velocity as the envelope moves to the right in the transverse propagation example.

Download 11.5MB, Quicktime Format

Download Quicktime Player from Apple.


2. Plasmon Printing

The minimum feature size that can be obtained using conventional projection optical lithography is determined by the diffraction limit. Plasmon printing is a new approach to lithographic printing that takes advantage of the resonantly enhanced optical intensity in optical near field of metallic nanoparticles, and which could enable printing of deep subwavelength features using conventional photoresist and simple visible or ultraviolet light sources.



Available Presentations:

Plasmon Waveguides
Plasmon Printing


Available Publications:

Plasmonic Modes of Annular Nanoresonators Imaged by Spectrally Resolved Cathodoluminescence
Carrie E. Hofmann, Ernst Jan R. Vesseur, Luke A. Sweatlock, Henri J. Lezec, F. Javier Garcia de Abajo, Albert Polman, and Harry A. Atwater
Nano Letters (2007)


Plasmonics: A shifting perspective
Domenico Pacifici
Nature Photonics (2007)


Highly confined photon transport in subwavelength metallic slot waveguides
Jennifer A. Dionne, Henri J. Lezec, and Harry A. Atwater
Nanoletters Vol. 6, Issue 9, pp. 1928-1932 (2006)


Plasmon slot waveguides: towards chip-scale propagation with subwavelength-scale localization
Jennifer A. Dionne, Luke A. Sweatlock, Albert Polman, and Harry A. Atwater
Physical Review B 73, 035407 (2006)


Planar metal plasmon waveguides: frequency-dependent dispersion, propagation, localization, and loss beyond the free electron model
Jennifer A. Dionne, Luke A. Sweatlock, Albert Polman, and Harry A. Atwater
Physical Review B 72, 075405 (2005)


Plasmonics: Localization and guiding of electromagnetic energy in metal/dielectric structures
Stefan A. Maier and Harry A. Atwater
Journal of Applied Physics (2005)


The New 'p-n Junction': Plasmonics Enables Photonic Access to the Nanoworld
Harry A. Atwater, Stefan Maier, Albert Polman, Jennifer A. Dionne, Luke A. Sweatlock
MRS Bulletin, pp 385-389 (2005)


Image resolution of surface-plasmon-mediated near-field focusing with planar metal films in three dimensions using finite-linewidth dipole sources
Pieter G. Kik, Stefan A. Maier, and Harry A. Atwater
Physical Review B (2004)


Local detection of electromagnetic energy transport below the diffraction limit in metal nanoparticle plasmon waveguides
Stefan A. Maier, Pieter G. Kik, Harry A. Atwater, Sheffer Meltzer, Elad Harel, Bruce E. Koel, and Ari A.G. Requicha
Nature Materials (2003)


Microwave Analogue to a Subwavelength Plasmon Switch
Luke A. Sweatlock, Stefan A. Maier, and Harry A. Atwater
Proceedings of Electronic Components and Technology Conference (2003)


Optical pulse propagation in metal nanoparticle chain waveguides
Stefan A. Maier, Pieter G. Kik, and Harry A. Atwater
Physical Review B (2003)


Electromagnetic energy transport along Yagi arrays
Stefan A. Maier, Mark L. Brongersma, Harry A. Atwater
Materials Science and Engineering C (2002)


Metal nanoparticle arrays for near field optical lithography
Pieter G. Kik, Andrea L. Martin, Stefan A. Maier, and Harry A. Atwater
Proceedings of SPIE 4810 (2002)


Observation of coupled plasmon-polariton modes in Au nanoparticle chain waveguides of different lengths: Estimation of waveguide loss
Stefan A. Maier, Pieter G. Kik, and Harry A. Atwater
Applied Physics Letters (2002)


Observation of coupled plasmon-polariton modes of plasmon waveguides for electromagnetic energy transport below the diffraction limit
Stefan A. Maier, Pieter G. Kik, Harry A. Atwater, Sheffer Meltzer, Ari A.G. Requicha, and Bruce E. Koel
Proceedings of SPIE 4810 (2002)


Observation of near-field coupling in metal nanoparticle chains using far-field polarization spectroscopy
Stefan A. Maier, Mark L. Brongersma, Pieter G. Kik, and Harry A. Atwater
Physical Review B 65, 193408 (2002)


Electromagnetic energy transport along arrays of closely spaced metal rods as an analogue to plasmonic devices
Stefan A. Maier, Mark L. Brongersma, and Harry A. Atwater
Applied Physics Letters (2001)


Plasmonics - A Route to Nanoscale Optical Devices
Stefan A. Maier, Mark L. Brongersma, Pieter G. Kik, Sheffer Meltzer, Ari A. G. Requicha, Bruce E. Koel, and Harry A. Atwater
Advanced Materials (2001)


Electromagnetic energy transfer and switching in nanoparticle chain arrays below the diffraction limit
Mark L. Brongersma, John W. Hartman, Harry A. Atwater
Physical Review B (2000)